Nature Communications

Reversible single crystal photochemistry and spin state switching in a metal-cyanide complex

2025-09-29

Manipulating the physical properties of solid matter using only photons is a major challenge in materials science. However, achieving such control over a chemical reaction in the solid state is even more challenging. Here we demonstrate the reversible photochemistry occurring in a single crystal of a simple cyanide complex, K 4 [Mo III (CN) 7 ]·2H 2 O. Upon exposure to visible light at different wavelengths, a reversible breaking and reformation of dative bonds is triggered, resulting in a photoswitching of the Mo III coordination geometry between 6- and 7-coordinate. This transformation, in turn, induces a spin state change. The observed solid-state photochemical reactivity is robust, quantitative and occurs at a record-high temperature. It paves the way for the development of new photo-switchable high-temperature magnets and nanomagnets.

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DOI https://doi.org/10.1038/s41467-025-63523-x