Thermodynamic phase transitions of nematic order in magnetic helices
- Zoey Tumbleson
- Sophie A. Morley
- Emily Hollingworth
- Arnab Singh
- Temuujin Bayaraa
- Nicolas G. Burdet
- Ahmad Us Saleheen
- Margaret R. McCarter
- David Raftrey
- Ronald J. Pandolfi
- Vincent Esposito
- Georgi L. Dakovski
- Franz-Josef Decker
- Alexander H. Reid
- Tadesse A. Assefa
- Peter Fischer
- Sinéad M. Griffin
- Stephen D. Kevan
- Frances Hellman
- Joshua J. Turner
- Sujoy Roy
2025-06-20
A nematic phase lacks translation order but has orientational order. Nematic phases have been discovered in a variety of systems, including liquid crystals, correlated materials, and superconductors. Here, we report on a magnetic nematic phase, where the basis components are composed of magnetic helices. We directly probed the order parameters associated with the magnetic helices using resonant soft x-ray scattering and find two distinct nematic phases with complex spatiotemporal signatures. Using x-ray correlation spectroscopy, we find that near the phase boundary between the two nematic phases, fluctuations coexist on multiple disparate timescales. Our micromagnetic simulations and density functional theory calculations show that the fluctuations occur concomitantly with a reorientation of the magnetic helices, indicating spontaneous symmetry breaking and the emergence of additional degrees of freedom. Our results provide a framework for characterizing exotic phases that can be extended to a broad class of physical systems.